450 Influence of clouds on the climate of the Earth
negatively to cloud feedback. It stands to reason, if all else remains the same, the
optical thickness of the cloud would be proportional to the vertically integrated
liquid water. Additionally, we may argue with Bohren (1985) that changes in the
microphysical properties of clouds would be produced due to changes in atmo-
spheric temperature and humidity. If the size of the cloud particles increases along
with liquid water content, the magnitude of the negative feedback would decrease.
Detailed modeling is required to resolve the remaining questions.
12.2.4 Climatic impact due to aerosols
As is well-known, atmospheric aerosols have a strong impact on the greenhouse
effect of the Earth–atmosphere system due to aerosol extinction in the short-wave
and long-wave parts of the spectrum. As in case of clouds, the resulting effects
depend strongly on the particle concentration, on the optical properties of the
particles, and on the vertical as well as on the horizontal aerosol distributions.
In general, the effect of increasing concentrations of aerosol particles results in an
increase of the planetary albedo. The resulting cooling may counteract the green-
house warming of CO
2
and other trace gases as pointed out by Hansen and Lacis
(1990) and by others.
The single scattering albedo ω
0
of the aerosol particles plays an important role
in the radiation budget of the atmosphere since the aerosol effect can switch from
cooling to heating when ω
0
crosses a certain critical value. Due to the complex
composition of aerosol particles, the complex index of refraction is difficult to
measure accurately which is a prerequisite for accurate Mie calculations of the
extinction parameters and the phase function.
The relatively small mass of stratospheric aerosols plays an important role in
the radiation budget because of their global distribution and their long lifetime.
Occasionally, volcanic eruptions increase the stratospheric aerosol concentration
over the whole globe for a period of years so that they are an important cause
for primary global climate forcing. The stratospheric aerosols, mostly sulfuric acid
particles, have a very small imaginary part of the complex index of refraction which
results in small values of the absorption coefficient. For an average global albedo
of about 30%, they contribute to global cooling. In the stratosphere itself, however,
the main effect of the aerosols is an increase of the stratospheric temperature due
to the slight absorption of the particles themselves and due to the increase of the
photon pathlength in the absorbing gases. This warming was observed after the
El Chichon eruption as reported by Labitzke et al. (1983). Therefore, the cooling
effect of the stratospheric aerosols is limited to the troposphere and to the surface.
Tropospheric aerosols have a much larger optical depth than stratospheric
aerosols. However, tropospheric aerosols have a relatively short residence time